Why can I not remove music and why are my purchased songs being duplicated each time I sync??

So I'm not sure if this is unique but I have a couple of things going on.
1st issue: I have a iphone 4s. Itunes on my desktop. Some music purchased from the desktop is on my iphone and I cannot remove it. I've checked "manually manage music". I've selected only the playlists I want. It will not delete the purchased music.
2nd issue: Each time I sync it pulls only the purchased music from my iphone and adds it to my music library. And each time it does that, it's adding another copy of the purchased songs into my music folder. I tried a variety of options, synced 7 times, and ended up with 7 copies of each purchased song. I've triedso many different things I'm thinking the only thing left is to do a reset. Or possibly reinstalling itunes completely. I've unchecked "copy files to itunes media folder when adding to library" and unchecked each of the songs from the library.Very frustrating!
Any suggestions would really be appreciated!

Thanks, randers4.
Unchecking the individual songs from the iTunes music library does indeed remove the songs from my iPhone. However, this is quite tedious given the number of albums I want to remove. Isn't this supposed to be easier done by "unchecking" the Genre or the specific Album using the Devices/My iPhone/Music tab?
Does this work for you (or anyone else)? My aim is to identify the most efficient method of doing this.
Thanks,
MLawson

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