Why can't i remove files from my iPhone?

I have audiobooks and music files on my iPhone and iPod that I would like to remove so that I can put new ones on and I cannot remove them in iTunes.  I never had this problem before iOS 5 and the latest update for iTunes.  I have tried clicking on the file and pressing the delete key and right clicking but the delete/remove option is no longer there.  I have searched the iTunes help file and cannot find any answers.  Does anyone know how to remove these files?  Thanks in advance for any help!

No one here knows why. No one can help you with so little information because we do not have a crystalball. You will need to provide detailed information about what happens when you try to buy an app in order to begin to help with your issue.

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