Why is Gmail SMTP server working for only one of two accounts?

iPhone 4S, with all updates.
I have two gmail accounts, primary and secondary. I have both accounts set to use smtp.gmail.com, with password authentication for each account.
Primary account can send just fine using SMTP. Secondary account cannot send through it's "own" server (i.e., [email protected]) and sent messages failover to the primary account server ([email protected]). Of course, that means recipients see the email as coming from the primary account, which is totally contrary to the reason I have it.
Settings for smtp are identical, except for username and password. I can send using the secondary account in Mail on my Mac, using that server, with messages showing properly (i.e. from [email protected]).
Any ideas what's going on?

On the iPhone that can't send or receive iMessages, make sure iMessage is On in Settings > Message.
Also, try the tips in this Apple doc -> iOS: Troubleshooting Messages
If you still can't send or receive iMessages
To send and receive iMessages, your device must have a valid cellular or Wi-Fi data connection.
iOS: Troubleshooting Wi-Fi networks and connections
iOS: Troubleshooting cellular data
Ensure that iMessage is turned on in Settings > Messages.
iMessage registration validates your Apple ID for use with iMessage. If you are unable to activate iMessage, follow this article.
If iMessage is unavailable either on the sending or receiving device, SMS will be used. You can turn this on or off in Settings > Messages > Send As SMS. Carrier messaging rates may apply.
Verify that the Apple ID or phone number is listed in Settings > Messages > Send & Receive.
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