Why will music that previously synced with phone no longer sync, stating not compatible?

Why would music that previously synced to my iPhone no longer sync, stating not compatible.  Had a 4s, 64 GB, that was almost filled to capacity, so when I first got this message I though maybe that had something to do with it.  However, I now have the iPhone 6, 128 GB, and get the same message.  This involves some music that synced to my 4s for 2 to 3 years, and 2 CDs that I downloaded onto my MacBook Pro and into my ITunes library that had also synced previously with no problem.  There may be other music involved also.  Haven't fully investigated the extent of what is not syncing.

Thank you for your reply,
I checked the songs, they work. The computer was authorized.
Here is another interesting thing, I went to my old computer, and everything syncs (but the library on that comp is old).
I just don't understand why the music won't transfer (because all the other info transfers just fine)
In the phone menu I have everything checked off properly such as (sync all music and playlists).
Hmm. Any other suggestions?

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