Why wont iTunes transfer certain files?

For example, I've downloaded some movies from iTunesU that show up as individual files (in folders) in the playlist. I can't drag or seemingly move this files. How do I get them to the phone?
Thanks.

Check that your Computer is Authorised...
Open iTunes
From the Store menu, choose Authorize This Computer. (In earlier versions of iTunes, access this option from the Advanced menu).
When prompted, enter your Apple ID and password, then click Authorize.
From Here
About authorization and deauthorization

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