You can't open the application Library because it may be damaged or incomplete

I am a newby to the support communities as a questioner though I have searched and found quite a few answers to other problems.  My problem today is the above message whenever I click on an .mp4 file in my Finder.  The files are in my iTunes Library and play just fine in iTunes.  I clicked on an .mp3 file in Finder and it took me right to iTunes and played the song. I tried the same test with a .pdf file and Adobe came up right away with the file.
This seems to have started when I noticed my new WD Book Live started prompting me that there was no valid SSL for the drive.  It only prompts me on my Mac Mini - iPhone and iPad are fine. I clicked to Trust Always for that drive and when I clicked on one of the movies, it says "No default application associated with the .mp4 file extension."  I cannot seem to find anything to do with file extensions in System Preferences or System Utilities.
Any suggestions anyone.  Much appreciated
Mac Mini 1.66 GHz Intel Core Duo
2 GB 667 GHz DDR2 SDRAM
Mac OS X 10.6.8
iTunes 11.1.5 (5)

Hello Brian,
Thank you for the details of the issue you are experiencing with opening .mp4 files from the Finder.  It sounds like you may need to set iTunes (or an alternate application that plays .mp4 files) as the default application to open .mp4 files on your computer. 
Use these steps:
To always open a document with a specific application:
In the Finder, select the document’s icon and choose File > Get Info.
In the Info window, click the disclosure triangle next to “Open with.”
Choose the application you want to use from the pop-up menu.
If you want all documents of this file type to open with the same application, click Change All.
In step 3, be sure to select iTunes (or an alternate application that plays .mp4 files) from the Applications folder on your computer.
Mac OS X 10.6: If a document doesn’t open with the right application
http://support.apple.com/kb/PH6767
Thank you for using Apple Support Communities.
Best,
Sheila M.

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