2 laptops, 2 libraries, home sharing but can't sync both libraries

My husband's laptop has 'home library'. My laptop has 'on this PC'. Through home sharing we can see all songs from both libraries, but I can't sync my ipod from 'home library' and he can't sync from 'on this PC' which has all the newly purchased songs. There must be a way to get access to all our combined songs. Help!

I was thinking I would need to do a new backup from his library and re-download purchased stuff.  (Making sure that I have deleted all previous backups on the external hard-drive to make sure I don't use the wrong one again!!)  As you have probably guessed I'm not that PC-savvy so I don't know if I would trust myself to paste it in the correct place.  Will set aside a couple of hours tomorrow to redo the backup and re-download the songs.
Thanks very much for your fast responses here. Much appreciated! Wish me luck

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