Made an error moving iTunes Music and need to create a folder ...

In August when I had to re-install iTunes, motherboard melt down, I thought I'd transferred iTunes Music back to the F drive, where I keep my media library, correctly.
All downloads installed there and when I clicked Add Folder from my backup drive it installed without incident so everything was correct, or so I thought.
Today I got around to doing a backup with Synctoy and found out I was wrong.
The movies, music, etc. are all on F but they're not in a folder!
So Synctoy returns : error could not read from the source file system volume information.\access is denied.
The solution should be to create a folder on F for all the files, about 500 GB, but how do I do this and still keep the path for iTunes to follow?
Given that error the backup is not reliable even though Synctoy did, apparently, do a full back up anyway.

I tried the same thing about 6 months ago. Unfortunately, the maestros at iTunes have created an annoying feature so that the iTunes library can ONLY be sited in your "My Music" folder on your internal hard drive.
From the iTunes help menu, "The iTunes Library file is a database of the songs and videos in your library and the playlists you've created. This file is located in the iTunes folder inside your My Music folder (in your My Documents folder). Do not move this file to another location. If you delete it, iTunes will create a new, empty copy the next time you open iTunes, but any playlists, song ratings, comments, or other information you created will be lost.
What a monumental bummer!!

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