Why can't I sync my iTunes Library from my second laptop to my iPod?

I just synced my iPod to my iTunes library on my OLD laptop and then used Home Sharing to import that content to my new laptop.
Then, I tried syncing my iTunes Library from my new laptop to my iPod and it said " This will delete all old music, videos & movies from your iPod and replace it with your iTunes Library" wich is exactly what I wanna do! So I clicked continue and it started syncing...
During the middle of the process a pop up appears and says " Your iTunes LIbrary cannot be synced to your iPod because there is not enough room on your iPod (additionaly 2.33GB required) "
But I thought it would erase my songs from my ipod ( approximately 2.40GBs) and replace it with the new ones from my library (2.33GB) ???? Why didn't it? What can I do to have my iTunes Library from my new laptop to my iPod Touch?
( I want my iPod to be able to sync anytime to my new computer because I'm getting rid of the old one.)
Please help, thanks.

So I copied everything in the iTunes folder from my old computer
and sent it to an 8GB USB,
which I'll insert into my new computer and paste the files on to /Music/
Will that work?

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