Using Multiple Hard Drives for iTunes Storage

I am running out of room on my current hard drive and want to use a new external hard drive to add space. My problem is I want to use both hard drives for storage (not the same music). Is this possible as I have only been able to direct iTunes to one hard drive? Thank you.
Dual G5   Mac OS X (10.4.5)   400GB Raid set

When you change the location in iTunes preferences what you are doing is telling iTunes where ripped music should be put. It isn't changing where iTunes should look for music that is already in the library. So go ahead and change the location to where you want music to be stored from now on. iTunes won't lose the other music. (At one times my iTunes library was spread over 4 drives.)

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