Using an old iPod as storage for part of my iTunes Library.

I have an old 4th Gen iPod (40gb) that needs a new battery, which I plan to have repaired. I know that i can use the iPod as a hard drive, however, as my iTunes Library has grown to a huge size (pushing 63Gb), it is taking up rather more of my MacBook Pro's Hard disk space, than I would like.
My question is this; Is there a way that I can store part of my iTunes music on the iPod and the rest on the Macbook Pro? Then, when i needed the full library, I would simply plug in my iPod/Hard drive. Is this possible? and also, would it be as straight forward as plugging in the iPod and launching iTunes?
Hope you can advise me.
Cheers

" I know that PCs don't recognise Mac stuff but, and correct me if I'm wrong, I remember something about Macs recognising PC stuff??"
An iPod formatted for Mac it won't run natively on a PC because the Windows OS does not support the HFS Plus file system and therefore will not see the drive. There are third party helper programs to overcome that, however Macs can read Windows formatted drives so you should be able to use your old iPod as a straightforward removable drive without any problem.

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