Inability to copy music from iTunes library to 4S

I'm having trouble copying music from my iTunes library (Windows PC running Vista). 
It copies three or four albums without any problems and the stops on the third or fourth track on the next album and returns an error message (iTunes cannot copy..... unknown error (-69)). 
When this happens, iTunes then slows the whole machine down - Internet Explorer stops responding, as does Windows Explorer, as well as most other programs  It's really frustrating. 
I don't know whether updating the OS to Windows 7 will remedy it, but it's an option.  I have the most up to date iTunes, Vista and iOS versions, so I'm stumped.  I might take the iPhone to a local reseller and see what they can suggest, but I thought I'd ask you guys first.

http://support.apple.com/kb/ht1210

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