My main library is stored in my G:drive, but can't remember how to open iTunes such that I can reselect/designate that library as the main, rather than my laptop temp library... any advice?

Just sorted.

Unfortunately I don't have first hand experience with the Lacie device but reading your question you said you installed the Seagate media app. I checked the App Store and there is also a LaCie app by Seagate. Check also the link below. I,m going to ask the hosts to move your question to the iPad Forum, hopefully someone has an answer for you.
LaCie Media by Seagate Technology https://appsto.re/us/XWzOZ.i
https://www.lacie.com/us/products/product.htm?id=10618

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